I think your proposed model may be inappropriate for your data. The main trend in your data is a simple exponential decay, whicha model that fits remarkably well:
nlm = NonlinearModelFit[data, beta Exp[-gamma t], {{beta, 1}, {gamma, 100}}, t]
Show[
LogLinearPlot[
Legended[nlm[t], "fit"], {t, data[[1, 1]], data[[-1, 1]]},
Frame -> True, Axes -> False,
PlotRange -> All,
PlotStyle -> Directive[Opacity[0.3, Blue], Thickness[0.02]]
],
ListLogLinearPlot[Legended[data, "data"], PlotStyle -> Black]
]
data
comes from data = ImportString[" your data table minus the headers ", "Table"]
.