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The requirement that la + lc == 100 is simple to implement, just pass 100 - la to Fc, or use ModelP/.{lc->100-la} in the call to FindFit. For the other trouble, remember that N is a special function in Mathematica, so avoid ever using this as a variable. Using n instead, I tried ModelP = (2/q^4)*Re[((1 - Fc[q, lc, sc])*(1 - Fa[q, la, sa]))/ (1 - ...

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