I think you mean something like this:
Clear[char];
{Slider[Dynamic[char], {67, 97, 1}], Dynamic[FromCharacterCode[char]]}
The syntax in your question was incorrect because the dynamic variable in the first argument of Slider can't be a protected function name.
Edit
You also had a ToExpression in your question. That can be added in this answer too, obviously by writing ToExpression@FromCharacterCode. Then you just have to make sure your character range doesn't include characters that yield an error when fed into ToExpression.
Edit 2
In response to the comment, I think what you should do is to write
a = Dynamic[ToExpression@FromCharacterCode[char]]
with the above slider (or some version of it).
afurther below but you should fix up this question describing whatais and how it relates tochar. – Mike Honeychurch Dec 5 '12 at 20:44